Fictional Characters with Mental Disabilities...

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[youtube]http://www.youtube.com/watch?v=jOcl8aUZ8J8[/youtube]
I'm pretty sure that Pterano has Narcissistic Personality Disorder, and that Sierra might have Antisocial Personality Disorder. I can't come up with a proper diagnosis for Rinkus.

John Rambo: PTSD - fought in the Vietnam War

Anakin Skywalker: Borderline Personality Disorder - almost always had uncontrollable emotional fits and constant negative self-talk

Roger the Alien: Sociopath - always seems to get himself into situations involving other people without considering the moral consequences

Jar Jar Binks: ADHD - he was aloof bugging Qui-Gon and unknowingly making a fool out of himself

Squidward: Narcissism and Depression - he has a whole easter island head house full of pictures that look like him and always admires himself; gets really sad about life in Bikini Bottom, working at the Krusty Krab and being around SpongeBob and Patrick; wishes he was dead

I don't know if any of these characters were previously mentioned but here are the ones I can think of.

Soul Eater
Death the Kid has a symmetry OCD.
Crona (or Chrona) has mild depression and an inferiority complex due to neglect and abuse from his/her mother. He/she is also rather antisocial.
Professor Stein is obviously insane.
Medusa, Crona's mother, probably has something. Haven't seen her enough to know what, though.

Bleach
Aizen has a god complex/wants to be a powerful immortal being.
Ulquiorra displays no emotion unless extremely provoked.
Kon most likely has ADHD/Aspergers.

Homestuck
Karkat has an inferiority complex.
John probably has ADHD or something similar.
Kankri most likely has troll Aspergers and maybe a superiority complex.
Mituna may have troll Tourettes and is mentally challenged (SPOILERS) after burning out his psionics.
Kurloz is selectively mute and sewed his own mouth shut, also has bad night-terrors.
Sollux is bipolar in relation to him being a Gemini.
Calliope and Caliborn are representative of multiple personality disorder because they both live in the same body.
Gamzee is crazy, may be bipolar or have MPD.
The Condesce is probably Narcissistic/Sociopath.

Edd from Ed, Edd n Eddy has OCD.

L from Deathnote with AS/HFA

Ray Babbitt from Rain Man- Autism

Lisa Simpson from The Simpsons- Aspergers Syndrome or HFA

Mr. Spock from Star Trek- Aspergers Syndrome or HFA

Peter Parker from Spider Man- Aspergers Syndrome

Gollum from The Lord Of The Rings- Tourettes Syndrome, Schiziophernia, or Bipolar Disorder

Dorothy Ann from The Magic School Bus- HFA

My version of Twilight Princess Link has PDD-NOS.

I'll add:

Carlos from The Magic School Bus- Narcissstic Personality Disorder

Arnold from The Magic School Bus- Aspergers Syndrome

Lady Mary from Downton Abbey- Narcisstic Personality Disorder

Trixie from Call The Midwife- Narcisstic Personality Disorder

Bruce Banner from The Incredible Hulk and The Avengers- HFA

Agent Fitz from Agents Of SHIELD- PDD NOS

Harold Finch from Person Of Interest- HFA

Root from Person of Interest- PDD NOS

IIRC, Benny Stulwicz from L.A. Law (Larry Drake) was also somewhat mentally ret*d.

Greece from Axis Powers Hetalia has autism-he's very quiet and withdrawn, and his special interest is cats.

(This is my headcanon because I have Asperger's, and Greece is my favorite, and I like characters with neurological disorders.)