Two-Face is one of my fave Batman villains, which was brilliantly done in the Long Halloween. Aaron Eckhart's incarnation s**ts all over Tommy Lee Jones's cackling bubblegum faced Joker reject from a great height. Also, the Arkham City Two-Face looks absolutely bad-arse.
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"I've seen things you people wouldn't believe: Attack ships on fire off the shoulder of Orion; I've watched c-beams glitter in the dark near the Tannhauser Gate. All those moments will be lost in time; like tears in rain. Time to die." Roy Batty